Magnetic structure of the antiferromagnetic half-Heusler compound NdBiPt

We present results of single crystal neutron diffraction experiments on the rare-earth, half-Heusler antiferromagnet (AFM) NdBiPt. This compound exhibits an AFM phase transition at $T_{\mathrm N}=2.18$~K with an ordered moment of $1.78(9)$~$μ_{\mathrm B}$ per Nd atom. The magnetic moments are aligned along the $[001]$-direction, arranged in a type-I AFM structure with ferromagnetic planes, alternating antiferromagnetically along a propagation vector $τ$ of $(100)$. The $R$BiPt ($R$= Ce-Lu) family of materials has been proposed as candidates of a new family of antiferromagnetic topological insulators (AFTI) with magnetic space group that corresponds to a type-II AFM structure where ferromagnetic sheets are stacked along the space diagonal. The resolved structure makes it unlikely, that NdBiPt qualifies as an AFTI.

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