Magnetic structure and magnon dispersion in LaSrFeO4_4

preprint2013arXivOpen access

Abstract

We present elastic and inelastic neutron scattering data on LaSrFeO4_4. We confirm the known magnetic structure with the magnetic moments lying in the tetragonal basal plane, but contrarily to previous reports our macroscopic and neutron diffraction data do not reveal any additional magnetic phase transition connected to a spin reorientation or to a redistribution of two irreducible presentations. Our inelastic neutron scattering data reveals the magnon dispersion along the main-symmetry directions [0 ξξ 0] and [ξξ -ξξ 0]. The dispersion can be explained within linear spin-wave theory yielding an antiferromagnetic nearest-neighbour interaction parameter J1=7.4(1)J_{1}=7.4(1) meV and a next-nearest neighbour interaction parameter J2=0.4(1)J_{2}=0.4(1) meV. The dispersion is gapped with the out-of-plane anisotropy gap found at Δout=5.26(2)Δ_{out}=5.26(2) meV, while evidence is present that the in-plane anisotropy gap lies at lower energies, where it cannot be determined due to limited instrument resolution.

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