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Magnetic field-modulated exciton generation in organic semiconductors: an intermolecular quantum correlation effect

Magnetoelectroluminescence (MEL) of organic semiconductor has been experimentally tuned by adopting blended emitting layer consisting of both hole and electron transporting materials. A theoretical model considering intermolecular quantum correlation is proposed to demonstrate two fundamental issues: (1) two mechanisms, spin scattering and spin mixing, dominate the two different steps respectively in the process of the magnetic field modulated generation of exciton; (2) the hopping rate of carriers determines the intensity of MEL. Calculation successfully predicts the increase of singlet excitons in low field with little change of triplet exciton population.

preprint2009arXivOpen access
B. F. DingY. YaoX. Y. SunZ. Y. SunX. D. GaoZ. T. XieZ. J. WangX. M. DingY. Z. WuX. F. JinC. Q. WuX. Y. Hou
cond-mat.mes-hallcond-mat.mtrl-sci
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Open access12 authors2 topics
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B. F. DingY. YaoX. Y. SunZ. Y. SunX. D. GaoZ. T. XieZ. J. WangX. M. DingY. Z. WuX. F. JinC. Q. WuX. Y. Hou

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