Magnetic-field-induced transition from metastable spin glass to possible antiferromagnetic-ferromagnetic phase separation in Cd0.5Cu0.5Cr2O4Cd_{0.5}Cu_{0.5}Cr_2O_4

preprint2008arXivOpen access

Abstract

Using ac susceptibility, dc magnetization and heat capacity measurements, we have investigated the magnetic properties of Cd0.5Cu0.5Cr2O4Cd_{0.5}Cu_{0.5}Cr_2O_4. Cd0.5Cu0.5Cr2O4Cd_{0.5}Cu_{0.5}Cr_2O_4 has an extraordinary magnetic phase including a metastable spin-glass(SG) phase at zero field, a possible phase separation scenario of AFM/FM above ∼0.5T\sim 0.5T field, and at intermediate fields, an apparent pseudo reentrant spin-glass (RSG) plateau is observed. These phenomena are closely correlated with the pinning effect of the Cu2+Cu^{2+} sublattice on the frustrated lattice.

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