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Magnetic excitations in L-edge resonant inelastic x-ray scattering from one-dimensional cuprates

We study the magnetic excitation spectra of L-edge resonant inelastic x-ray scattering (RIXS) from the spin singlet ground state in one-dimensional undoped cuprates. Analyzing the transition amplitudes of the magnetic excitations in the second-order dipole allowed process, we find that the magnetic excitations are brought about not only on the core-hole site but also on the neighboring sites. The RIXS spectra are expressed by the one-spin correlation function in the scattering channel with changing polarization, and the two-spin correlation function in the scattering channel without changing polarization. The latter could not be brought about within the so-called UCL approximation. We calculate these correlation functions on a finite-size ring. An application to the possible RIXS spectra in Sr_2CuO_3 demonstrates that the contribution of the two-spin correlation function could be larger than that of the one-spin correlation function in the σpolarization for the momentum transfer around the zone center.

preprint2011arXivOpen access

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