Magnetic and Electronic Properties of Spin-Orbit Coupled Dirac Electrons on a (001)(001) Thin Film of Double Perovskite Sr2_2FeMoO6_6

preprint2020arXivOpen access

Abstract

We present an interacting model for the electronic and magnetic behavior of a strained (001)(001) atomic layer of Sr2_2FeMoO6,_6, which shows room-temperature ferrimagnetism and magnetoresistance with potential spintronics application in the bulk. We find that the strong spin-orbit coupling in the molybdenum 4dd shell gives rise to a robust ferrimagnetic state with an emergent spin-polarized electronic structure consisting of flat bands and four massive or massless Dirac dispersions. Based on the spin-wave theory, we demonstrate that the magnetic order remains intact for a wide range of doping, leading to the possibility of exploring flat band physics, such as Wigner crystallization in electron-doped Sr2−x_{2-x}Lax_{x}FeMoO6._6.

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