Macroscopic Anisotropy and Symmetry Breaking in the Pyrochlore Antiferromagnet Gd2_{2}Ti2_{2}O7_{7}}

preprint2002arXivOpen access

Abstract

In the Heisenberg antiferromagnet Gd2Ti2O7Gd_2Ti_2O_7, the exchange interactions are geometrically frustrated by the pyrochlore lattice structure. This ESR study reveals a strong temperature dependent anisotropy with respect to a [111] body diagonal below a temperature TA=80T_A=80 K, despite the spin only nature of the Gd3+Gd^{3+} ion. Anisotropy and symmetry breaking can nevertheless appear through the superexchange interaction. The presence of short range planar correlation restricted to specific Kagomé planes is sufficient to explain the two ESR modes studied in this work.

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