Long-range plasmon-assisted energy transfer over doped graphene

preprint2012arXivOpen access

Abstract

We demonstrate that longitudinal plasmons in doped monolayer graphene can mediate highly efficient long-range energy transfer between nearby fluorophores, e.g., semiconductor quantum dots. We derive a simple analytical expression for the energy transfer efficiency that incorporates all the essential processes involved. We perform numerical calculations of the transfer efficiency for a pair of PbSe quantum dots near graphene for inter-fluorophore distances of up to 1 μμm and find that the plasmon-assisted long-range energy transfer can be enhanced by up to a factor of ∼104\sim10^4 relative to the Förster's transfer in vacuum.

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