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Lattice-Tuned Magnetism of Ru4+(4d4) Ions in Single-Crystals of the Layered Honeycomb Ruthenates: Li2RuO3 and Na2RuO3

We synthesize and study single crystals of the layered honeycomb lattice Mott insulators Na2RuO3 and Li2RuO3 with magnetic Ru4+(4d4) ions. The newly found Na2RuO3 features a nearly ideal honeycomb lattice and orders antiferromagnetically at 30 K. Single-crystals of Li2RuO3 adopt a honeycomb lattice with either C2/m or more distorted P21/m below 300 K, depending on detailed synthesis conditions. We find that Li2RuO3 in both structures hosts a well-defined magnetic state, in contrast to the singlet ground state found in polycrystalline Li2RuO3. A phase diagram generated based on our results uncovers a new, direct correlation between the magnetic ground state and basal-plane distortions in the honeycomb ruthenates.

preprint2014arXivOpen access
J. C. WangJ. TerzicT. F. QiFeng YeS. J. YuanS. AswarthamS. V. StreltsovD. I. KhomskiiR. K. KaulG. Cao
cond-mat.str-el
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J. C. WangJ. TerzicT. F. QiFeng YeS. J. YuanS. AswarthamS. V. StreltsovD. I. KhomskiiR. K. KaulG. Cao

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