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Interplay of thermal and quantum spin fluctuations on the kagome lattice

We present a Raman spectroscopic investigation of the Herbertsmithite ZnCu3(OH)6Cl2, the first realization of a Heisenberg s=1/2 antiferromagnet on a perfect kagome lattice. The magnetic excitation spectrum of this compound is dominated by two components, a high temperature quasi elastic signal and a low temperature, broad maximum. The latter has a linear low energy slope and extends to high energy. We have investigated the temperature dependence and symmetry properties of both signals. Our data agree with previous calculations and point to a spin liquid ground state.

preprint2010arXivOpen access
Dirk WulferdingPeter LemmensPatric ScheibJens RoederPhilippe MendelsMark A. de VriesShaoyan ChuTianheng HanYoung S. Lee
cond-mat.str-el
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Open access9 authors1 topic
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Dirk WulferdingPeter LemmensPatric ScheibJens RoederPhilippe MendelsMark A. de VriesShaoyan ChuTianheng HanYoung S. Lee

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