Interplay of magnetism, Fermi surface reconstructions, and hidden-order in the heavy-fermion material URu2_2Si2_2

preprint2012arXivOpen access

Abstract

URu2_2Si2_2 is surely one of the most mysterious of the heavy-fermion compounds. Despite more than twenty years of experimental and theoretical works, the order parameter of the transition at T0=17.5T_0 = 17.5 K is still unknown. The state below T0T_0 remains called "hidden-order phase" and the stakes are still to identify the energy scales driving the system to this phase. We present new magnetoresistivity and magnetization measurements performed on very-high-quality single crystals in pulsed magnetic fields up to 60 T. We show that the transition to the hidden-order state in URu2_2Si2_2 is initially driven by a high-temperature crossover at around 40-50 K, which is a fingerprint of inter-site electronic correlations. In a magnetic field H\mathbf{H} applied along the easy-axis c\bf{c}, the vanishing of this high-temperature scale precedes the polarization of the magnetic moments, as well as it drives the destabilization of the hidden-order phase. Strongly impurity-dependent magnetoresistivity confirms that the Fermi surface is reconstructed below T0T_0 and is strongly modified in a high magnetic field applied along c\mathbf{c}, i.e. at a sufficiently-high magnetic polarization. The possibility of a sharp crossover in the hidden-order state controlled by a field-induced change of the Fermi surface is pointed out.

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