Internal conversion of nuclear transition in the 235mU@C60−nXn{}^{235m}U@C_{60-n}X_n molecules and related compounds

preprint2010arXivOpen access

Abstract

The internal conversion of nuclear transition in the 235U{}^{235}U atom is considered. The low-energy γ−γ-quanta (Eγ≈E_γ \approx 76.8 eVeV) are emitted during the E3−E3-transition from the excited state (I=(12)+I = (\frac12)^+) of the 235U{}^{235}U nucleus to its ground state (I=(72)−I = (\frac72)^-). The decay rate of this 235mU{}^{235m}U isomer (E≈76.8E \approx 76.8 eVeV) noticeably depends upon the chemical composition and actual physical conditions (i.e. temperature TT and pressure pp). By varying such a composition and physical conditions one can change the life-time of the 235mU{}^{235m}U isomer to relatively large/small values. A specific attention is given to the fullerene molecules containing the central 235U{}^{235}U atom. It is shown that the decay rate λλ of the 235mU{}^{235m}U isomer in the 235mU@C60−nXn{}^{235m}U@C_{60-n}X_n molecules and related compounds can differ significantly from the values obtained for isolated 235U{}^{235}U atoms. Some applications of this effect are considered.

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