Indication for the coexistence of closed orbit and quantum interferometer with the same cross section in the organic metal (ET)4(H3O)[Fe(C2O4)3].C6H4Cl2: Persistence of SdH oscillations above 30 K

preprint2009arXivOpen access

Abstract

Shubnikov-de Haas (SdH) and de Haas-van Alphen (dHvA) oscillations spectra of the quasi-two dimensional charge transfer salt ββ"-(ET)4_4(H3_3O)[Fe(C2_2O4_4)3_3]⋅\cdotC6_6H4_4Cl2_2 have been investigated in pulsed magnetic fields up to 54 T. The data reveal three basic frequencies Fa_a, Fb_b and Fb−a_{b - a}, which can be interpreted on the basis of three compensated closed orbits at low temperature. However a very weak thermal damping of the Fourier component Fb_b, with the highest amplitude, is evidenced for SdH spectra above about 6 K. As a result, magnetoresistance oscillations are observed at temperatures higher than 30 K. This feature, which is not observed for dHvA oscillations, is in line with quantum interference, pointing to a Fermi surface reconstruction in this compound.

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