Incommensurate-Commensurate Magnetic Phase Transition in SmRu2_{2}Al10_{10}

preprint2015arXivOpen access

Abstract

Magnetic properties of single crystalline SmRu2_{2}Al10_{10} have been investigated by electrical resistivity, magnetic susceptibility, and specific heat. We have confirmed the successive magnetic phase transitions at TN=12.3T_{\text{N}}=12.3 K and TM=5.6T_{\text{M}}=5.6 K. Resonant x-ray diffraction has also been performed to study the magnetic structures. Below TNT_{\text{N}}, the Sm3+^{3+} moments order in an incommensurate structure with q1=(0,0.759,0)q_1=(0, 0.759, 0). The magnetic moments are oriented along the orthorhombic bb axis, which coincides with the magnetization easy axis in the paramagnetic phase. A very weak third harmonic peak is also observed at q3=(0,0.278,0)q_3=(0, 0.278, 0). The transition at TMT_{\text{M}} is a lock-in transition to the commensurate structure described by q1=(0,0.75,0)q_1=(0, 0.75, 0). A well developed third harmonic peak is observed at q3=(0,0.25,0)q_3=(0, 0.25, 0). From the discussion of the magnetic structure, we propose that the long-range RKKY interaction plays an important role, in addition to the strong nearest neighbor antiferromagnetic interaction.

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