Paper detail

Highly photo-stable, kHz-repetition-rate, diode pumped circulation-free liquid dye laser with thermal lens management

Liquid dye lasers have long been considered as ideal tunable laser sources in the visible range but are bulky, expensive, and require a complex system for dye circulation. Here, we present a system that relies on a low-cost blue laser diode as the pump source and a sealed dye cell with no flowing circuitry, resulting in a device that combines the convenience and size of a solid-state device with the stability of a liquid organic laser. A very high photo-stability is obtained (up to 1.2 x 10$^9$ pulses or 12 days at 1 kHz), which is five orders of magnitude higher than a solid-state dye laser operated in similar conditions. The number of pulses obtainable at low repetition rates is found to be limited by molecular self-diffusion and, hence, related to the total cuvette volume. In contrast, the repetition rate is limited to a few kHz, which suggests that thermal effects play a bigger role than triplet population effects. Thermal effects participate in the suppression of lasing through the buildup of a strong negative thermal lens; correcting the non-aberrant part of this thermal lens by resonator design enables the repetition rate to be pushed up to 14 kHz with possible further optimization. This work shows a route for building off-the-shelf, compact, low-cost, and convenient tunable pulsed lasers in the visible range that have superior stability over organic solid-state lasers.