Highly-confined spin-polarized two-dimensional electron gas in SrTiO3_{3}/SrRuO3_{3} superlattices

preprint2012arXivOpen access

Abstract

We report first principles characterization of the structural and electronic properties of (SrTiO3_{3})5_{5}/(SrRuO3_{3})1_{1} superlattices. We show that the system exhibits a spin-polarized two-dimensional electron gas, extremely confined to the 4dd orbitals of Ru in the SrRuO3_{3} layer. Every interface in the superlattice behaves as a minority-spin half-metal ferromagnet, with a magnetic moment of μμ = 2.0 μBμ_{\rm B}/SrRuO3_{3} unit. The shape of the electronic density of states, half metallicity and magnetism are explained in terms of a simplified tight-binding model, considering only the t2gt_{2g} orbitals plus (i) the bi-dimensionality of the system, and (ii) strong electron correlations.

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