High-order harmonic generation from Rydberg states at fixed Keldysh parameter

preprint2013arXivOpen access

Abstract

Because the commonly adopted viewpoint that the Keldysh parameter γγ determines the dynamical regime in strong field physics has long been demonstrated to be misleading, one can ask what happens as relevant physical parameters, such as laser intensity and frequency, are varied while γγ is kept fixed. We present results from our one- and fully three-dimensional quantum simulations of high-order harmonic generation (HHG) from various bound states of hydrogen with nn up to 40, where the laser intensities and the frequencies are scaled from those for n=1n=1 in order to maintain a fixed Keldysh parameter γγ<1< 1 for all nn. We find that as we increase nn while keeping γγ fixed, the position of the cut-off scales in well defined manner. Moreover, a secondary plateau forms with a new cut-off, splitting the HHG plateau into two regions. First of these sub-plateaus is composed of lower harmonics, and has a higher yield than the second one. The latter extends up to the semiclassical Ip+3.17UpI_p+3.17U_p cut-off. We find that this structure is universal, and the HHG spectra look the same for all n≳10n\gtrsim 10 when plotted as a function of the scaled harmonic order. We investigate the nn-, ll- and momentum distributions to elucidate the physical mechanism leading to this universal structure.

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