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High energy photoelectron emission from gases using plasmonics enhanced near-fields

We study theoretically the photoelectron emission in noble gases using plasmonic enhanced near-fields. We demonstrate that these fields have a great potential to generate high energy electrons by direct mid-infrared laser pulses of the current femtosecond oscillator. Typically, these fields appear in the surroundings of plasmonic nanostructures, having different geometrical shape such as bow-ties, metallic waveguides, metal nanoparticles and nanotips, when illuminated by a short laser pulse. In here, we consider metal nanospheres, in which the spatial decay of the near-field of the isolated nanoparticle can be approximated by an exponential function according to recent attosecond streaking measurements. We establish that the strong nonhomogeneous character of the enhanced near-field plays an important role in the above threshold ionization (ATI) process and leads to a significant extension in the photoelectron spectra. In this work, we employ the time dependent Schrödinger equation in reduced dimensions to calculate the photoelectron emission of xenon atoms in such enhanced near-field. Our findings are supported by classical calculations.

preprint2013arXivOpen access

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