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Ground state of the spin-1/2 chain of green dioptase at high fields

The gem-stone dioptase Cu6Si6O18.6H2O has a chiral crystal structure of equilateral triangular helices consisting of Cu-3d spins. It shows an antiferromagnetic order with an easy axis along c at TN = 15.5 K under zero field, and a magnetization jump at HC = 13.5 T when the field is applied along c-axis. By 29Si-NMR measurements, we have revealed that the high-field state is essentially the two sub-lattice structure, and that the component within ab-plane is collinear. The result indicates no apparent match with the geometrical pattern of helical spin chain.

preprint2013arXivOpen access
Kazuki MatsuiMasashi FujisawaKenta HagiwaraYukihiro HoshinoTakayuki GotoTakahiko SasakiHidekazu TanakaSusumu OkuboHitoshi Ohta
cond-mat.str-elcond-mat.mtrl-sci
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Kazuki MatsuiMasashi FujisawaKenta HagiwaraYukihiro HoshinoTakayuki GotoTakahiko SasakiHidekazu TanakaSusumu OkuboHitoshi Ohta

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