Abstract
As one of the primordial radioactive isotopes, Th mainly undergoes -decay with a half-life of yr. However, it is also one of 35 double beta decay candidates in which the single -decay is forbidden or strongly suppressed. 181 mg of thorium contained in a gas mantle was measured in an HPGe well-detector at the Gran Sasso Underground Laboratory (LNGS) with a total exposure of 3.25 g d. We obtain half-life limits on all double beta decay modes of Th to excited states of U on the order of yr. For the most likely transition into the state we find a lower half-life limit of yr (90% credibility). These are the first constraints on double beta decay excited state transition in Th.
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