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Ferromagnetism in CaRuO3 thin films by efficient route of tensile epitaxial strain

We show that a ferromagnetic (FM) order in the orthorhombic CaRuO3, which is a non-magnetic and iso-structural analog of FM system SrRuO3, can be established and stabilized by the means of tensile epitaxial strain. Investigations on the structural and magnetic property correlations in the CaRuO3 films with different degrees of strain reveal that the FM moment increases with increasing the tensile strain. This is an experimental verification to the theoretical predictions of scaling of the tensile epitaxial strain and the magnetic order in this system. Our studies further establish that the tensile strain is more efficient than the chemical route to induce the FM order in CaRuO3 as the magnetic moment in these strained films is larger than that in chemically modified CaRu0.9Cr0.1O3 films.