Fermi Surface of Metallic V2_2O3_3 from Angle-Resolved Photoemission: Mid-level Filling of egπe_g^π Bands

preprint2016arXivOpen access

Abstract

Using angle resolved photoemission spectroscopy (ARPES) we report the first band dispersions and distinct features of the bulk Fermi surface (FS) in the paramagnetic metallic phase of the prototypical metal-insulator transition material V2_2O3_3. Along the cc-axis we observe both an electron pocket and a triangular hole-like FS topology, showing that both V 3dd a1ga_{1g} and egπe_g^π states contribute to the FS. These results challenge the existing correlation-enhanced crystal field splitting theoretical explanation for the transition mechanism and pave the way for the solution of this mystery.

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