ESR of coupled spin-1/2 chains: unveiling zig-zag-type interchain correlations

By means of electron spin resonance investigations we revealed the crucial role of the interchain coupling in the spin dynamics of the spin-1/2 Heisenberg antiferromagnetic (AF) chain material copper-pyrazine-dinitrate, Cu(C$_4$H$_4$N$_2$)(NO$_3$)$_2$. We found that the dominating interchain interaction is of a zig-zag type. This interaction gives rise to geometrical frustration effects and strongly influences the character of AF ordering. Combining our experimental findings with the results of a quasiclassical approach we argue that at low temperatures the system orders in an incommensurate spiral state.

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