Abstract

In general, magnetism and superconductivity are antagonistic to each other. However, there are several families of superconductors, in which superconductivity may coexist with magnetism, and only a few examples are known, when superconductivity itself induces spontaneous magnetism. The most known compounds are Sr2_2RuO4_4 and some noncentrosymmetric superconductors. Here, we report the finding of a narrow dome of a novel s+is′s+is' superconducting (SC) phase with broken time-reversal symmetry (BTRS) inside the broad ss-wave SC region of the centrosymmetric multiband superconductor Ba1−x_{\rm 1-x}Kx_{\rm x}Fe2_2As2_2 (0.7≲x≲0.850.7 \lesssim x \lesssim 0.85). We observe spontaneous magnetic fields inside this dome using the muon spin relaxation (μμSR) technique. Furthermore, our detailed specific heat study reveals that the BTRS dome appears very close to a change in the topology of the Fermi surface (Lifshitz transition). With this, we experimentally demonstrate the emergence of a novel quantum state due to topological changes of the electronic system.

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