Electronic structure, optical and magnetic properties of Co2_{2}FeGe Heusler alloy films

preprint2012arXivOpen access

Abstract

Optical properties of ferromagnetic half-metallic full-Heusler Co2_{2}FeGe alloy are investigated experimentally and theoretically. Co2_{2}FeGe thin films were obtained by DC magnetron sputtering and show the saturation magnetization at TT=10 K of m≈m\approx5.6 μBμ_{B}/f.u., close to the value predicted by the Slater-Pauling rule. First-principles calculations of the electronic structure and the dielectric tensor are performed using the full-potential linearized-augmented-plane-wave method in the generalized gradient (GGA) and GGA+U approximations. The measured interband optical conductivity spectrum for the alloy exhibits a strong absorption band in the 1 - 4 eV energy range with pronounced fine structure, which agrees well with the calculated half-metallic spectrum of the system, suggesting a near perfect spin-polarization in the material.

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