Elastic Response in the Dilute non-Kramers System Y1−x_{1-x}Prx_xIr2_2Zn20_{20}

preprint2019arXivOpen access

Abstract

Ultrasonic investigations of the single-site quadrupolar Kondo effect in diluted Pr system Y0.966_{0.966}Pr0.034_{0.034}Ir2_2Zn20_{20} are reported. The elastic constant (C11−C12)/2(C_{11}-C_{12})/2 is measured down to ~40 mK using ultrasound for the dilute system Y0.966_{0.966}Pr0.034_{0.034}Ir2_2Zn20_{20} and the pure compound YIr2_2Zn20_{20}. We found that the elastic constant (C11−C12)/2(C_{11}-C_{12})/2 of the Pr-dilute system exhibits a logarithmic temperature dependence below T0T_0 ~0.3 K, where non-Fermi-liquid (NFL) behavior in the specific heat and electrical resistivity is observed. This logarithmic temperature variation manifested in the Γ3Γ_3-symmetry quadrupolar susceptibility is consistent with the theoretical prediction of the quadrupolar Kondo effect by D. L. Cox. On the other hand, the pure compound YIr2_2Zn20_{20} without 4f4f-electron contributions shows nearly no change in its elastic constants evidencing negligible phonon contributions. In addition, clear acoustic de Haas-van Alphen (dHvA) oscillations in the elastic constant were detected for both compounds on applying magnetic field. This is mainly interpreted as contribution from the Fermi surface of YIr2_2Zn20_{20}.

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