Doping-dependent bandwidth renormalization and spin-orbit coupling in (Sr1−x_{1-x}Lax_x)2_2RhO4_4

preprint2015arXivOpen access

Abstract

We investigate the electronic structure of (Sr1−x_{1-x}Lax_x)2_2RhO4_4 using a combination of the density functional and dynamical mean-field theories. Unlike the earlier local density approximation plus Hubbard UU (LDA+U) studies, we find no sizable enhancement of the spin-orbit splitting due to electronic correlations and show that such an enhancement is a spurious effect of the static mean-field approximation of the LDA+U method. The electron doping suppresses the importance of electronic correlations, which is reflected in quasi-particle bandwidth increasing with xx. (Sr1−x_{1-x}Lax_x)2_2RhO4_4 can be classified as weakly correlated metal, which becomes an itinerant in-plane ferromagnet (but possibly A-type antiferromagnet) due to Stoner instability around x=0.2x=0.2.

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