Abstract

Quasi-fission is the primary reaction mechanism that prevents the formation of superheavy elements in heavy-ion fusion experiments. Employing the time-dependent density functional theory approach we study quasi-fission in the systems 40,48^{40,48}Ca+238^{238}U. Results show that for 48^{48}Ca projectiles the quasi-fission is substantially reduced in comparison to the 40^{40}Ca case. This partly explains the success of superheavy element formation with 48^{48}Ca beams. For the first time, we also calculate the repartition of excitation energies of the two fragments in a dynamic microscopic theory. The system is found in quasi-thermal equilibrium only for reactions with 40^{40}Ca. The differences between both systems are interpreted in terms of initial neutron to proton asymmetry of the colliding partners.

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