Direct measurement of temporal correlations above the spin-glass transition by coherent resonant magnetic x-ray spectroscopy

In the 1970s a new paradigm was introduced that interacting quenched systems, such as a spin-glass, have a phase transition in which long time memory of spatial patterns is realized without spatial correlations. The principal methods to study the spin-glass transition, besides some elaborate and elegant theoretical constructions, have been numerical computer simulations and neutron spin echo measurements . We show here that the dynamical correlations of the spin-glass transition are embedded in measurements of the four-spin correlations at very long times. This information is directly available in the temporal correlations of the intensity, which encode the spin-orientation memory, obtained by the technique of resonant magnetic x-ray photon correlation spectroscopy (RM- XPCS). We have implemented this method to observe and accurately characterize the critical slowing down of the spin orientation fluctuations in the classic metallic spin glass alloy Cu(Mn) over time scales of 1 to 1000 secs. Our method opens the way for studying phase transitions in systems such as spin ices, and quantum spin liquids, as well as the structural glass transition.

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