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Diffusion transport coefficients for granular binary mixtures at low density. Thermal diffusion segregation

The mass flux of a low-density granular binary mixture obtained previously by solving the Boltzmann equation by means of the Chapman-Enskog method is considered further. As in the elastic case, the associated transport coefficients $D$, $D_p$ and $D'$ are given in terms of the solutions of a set of coupled linear integral equations which are approximately solved by considering the first and second Sonine approximations. The diffusion coefficients are explicitly obtained as functions of the coefficients of restitution and the parameters of the mixture (masses, diameters and concentration) and their expressions hold for an arbitrary number of dimensions. In order to check the accuracy of the second Sonine correction for highly inelastic collisions, the Boltzmann equation is also numerically solved by means of the direct simulation Monte Carlo (DSMC) method to determine the mutual diffusion coefficient $D$ in some special situations (self-diffusion problem and tracer limit). The comparison with DSMC results reveals that the second Sonine approximation to $D$ improves the predictions made from the first Sonine approximation. We also study the granular segregation driven by a uni-directional thermal gradient. The segregation criterion is obtained from the so-called thermal diffusion factor $Λ$, which measures the amount of segregation parallel to the temperature gradient. The factor $Λ$ is determined here by considering the second-order Sonine forms of the diffusion coefficients and its dependence on the coefficients of restitution is widely analyzed across the parameter space of the system. The results obtained in this paper extend previous works carried out in the tracer limit (vanishing mole fraction of one of the species) by some of the authors of the present paper.