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Crossover from charge order to strain glass in phase separated manganite thin films: Impact of thermal cycling and substrate induced strain

The magnetic and magnetotransport properties of single crystalline La1-x-yPryCaxMnO3 (x=0.42, y=0.40) thin films (~140 nm) deposited on (110) oriented LaAlO3 and SrTiO3 substrates exhibit a crossover from the high temperature antiferromagnetic-charge ordered insulator (AFM-COI) phase (T>TN) to strain glass (T<Tg). At intermediate temperatures (Tg<T<TN) dynamical liquid having prominent thermal-magneto-resistive hysteresis dominates in the cooling cycle, while in the warming cycle it is preceded by ferromagnetic metal (FMM) phase. Magnetic field required to drive AFM-COI to FMM phase transition are higher than that for the strain glass. The magneto-electric nature and temperature span of the distinct magnetic regimes are sensitive to the thermal cycling and substrate induced strain.

preprint2014arXivOpen access
Vasudha AgarwalP. K. SiwachV. P. S. AwanaH. K. Singh
cond-mat.mtrl-sci
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Vasudha AgarwalP. K. SiwachV. P. S. AwanaH. K. Singh

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