Confinement, reduced entanglement, and spin-glass order in a random quantum spin-ice model

preprint2019arXivOpen access

Abstract

We study an effective spin model derived perturbatively from random transverse-field Ising model on the pyrochlore lattice. The model consists of spin-configurations on the pyrochlore lattice, restricted to the spin-ice subspace, with spins interacting with random Ising exchange couplings as well as ring exchanges along the hexagons of the lattice. This model is studied by exact diagonalization upto N=64 site systems. We calculate spin-glass correlation functions and local entanglement entropy STS_T between spins in a single tetrahedron and the rest of the system. We find that the model undergoes two phase transitions. At weak randomness the model is in a quantum spin-ice phase where ST=ln⁡6S_T=\ln{6}. Increasing randomness first leads to a frozen phase, with long-range spin-glass order and ST=ln⁡2S_T=\ln{2} corresponding to the Cat states associated with Ising order. Further increase in randomness leads to a random resonating-hexagon phase with a frozen backbone of spins and a broad distribution of entanglement entropies. The implications of these studies for non-Kramers rare-earth pyrochlores are discussed.

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