Bulk domain Meissner state in the ferromagnetic superconductor EuFe2_{2}(As0.8_{0.8}P0.2_{0.2})2_{2}: Consequence of compromise between ferromagnetism and superconductivity

preprint2022arXivOpen access

Abstract

Small-angle neutron scattering (SANS) measurements are performed on the ferromagnetic superconductor EuFe2_{2}(As0.8_{0.8}P0.2_{0.2})2_{2} (Tsc=22.5 T\rm_{sc}=22.5\,K) to probe the delicate interplay between ferromagnetism and superconductivity. A clear signature of large ferromagnetic domains is found below the ferromagnetic ordering temperature TCT\rm_{C} = 18.5 K. In a small temperature interval of ∼\sim 1.5 K below TCT\rm_{C}, additional SANS signal is observed, of which the indirect Fourier transform reveals characteristic length scales in between ∼\sim 80 nm to ∼\sim 160 nm. These nanometer-scaled domain structures are identified to result from an intermediate inhomogeneous Meissner effect denoted domain Meissner state, which was recently observed on the surface of EuFe2_{2}(As0.79_{0.79}P0.21_{0.21})2_{2} crystals by means of magnetic force microscopy [V. S. Stolyarov et\mathit{et} al.\mathit{al.}, Sci. Adv. 4, 1061 (2018)], ascribing to the competition between ferromagnetism and superconductivity. Our measurements clearly render the domain Meissner state as a bulk phenomenon and provide a key solution to the mystery regarding the intriguing coexistence of strong ferromagnetism and bulk superconductivity in these compounds.

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