Antiferromagnetism in the magnetoelectric effect single crystal LiMnPO4_4

preprint2009arXivOpen access

Abstract

Elastic and inelastic neutron scattering studies reveal details of the antiferromagnetic tansition and intriguing spin-dynamics in the magneto-electric effect single crystal LiMnPO4_4. The elastic scattering studies confirm the system is antiferromagnetic (AFM) below TNT_N=33.75 K with local magnetic moments (Mn2+^{2+}; S=5/2S = 5/2) that are aligned along the crystallographic a-axis. The spin-wave dispersion curves propagating along the three principal axes, determined by inelastic scattering, are adequately modeled in the linear spin-wave framework assuming a spin-Hamiltonian that is parameterized by inter- and in-plane nearest- and next-nearest-neighbor interactions, and by easy-plane anisotropy. The temperature dependence of the spin dynamics makes this an excellent model many-body spin system to address the question of the relationship between spin-wave excitations and the order parameter.

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