Abstract
The double-perovskite ABB'O with heavy transition metal ions on the ordered B' sites is an important family of compounds to study the interplay between electron correlation and spin-orbit coupling (SOC). Here we prepared high-quality SrMgReO powder and single-crystal samples and performed non-resonant and resonant synchrotron x-ray diffraction experiments to investigate its magnetic ground state. By combining the magnetic susceptibility and heat capacity measurements, we conclude that SrMgReO exhibits a layered antiferromagnetic (AF) order at temperatures below 55 K with a propagation vector q = (001), which contrasts the previously suspected spin glass state. Our works clarify the magnetic order in SrMgReO and demonstrate it as a candidate system to look for magnetic octupolar orders and exotic spin dynamics.
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