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A multi-stop time-of-flight spectrometer for the measurement of positron annihilation-induced electrons in coincidence with the Doppler-shifted annihilation gamma photon

Here we describe an advanced multi functional, variable-energy positron beam system capable of measuring the energies of multiple positron-induced electrons in coincidence with the Doppler-shifted gamma photon resulting from the annihilation of the correlated positron. The measurements were carried out using the unique characteristics of the digital time-of-flight spectrometer and the gamma spectrometer available with the advanced positron beam system. These measurements have resulted in (i) the first digital time of flight spectrum of positron annihilation-induced Auger electrons generated using coincident signals from a high-purity Ge detector and a micro-channel plate; (ii) a two-dimensional array of the energy of Doppler-broadened annihilation gamma and the time of flight of positron-annihilation induced Auger electrons or secondary electrons measured in coincidence with the annihilation gamma photon; and (iii) the time of flight spectra of multiple secondary electrons ejected from a bilayer graphene surface as a result of the impact and(or) annihilation of positrons. The novelty of the gamma electron coincidence spectroscopy has been demonstrated by extracting the Doppler-broadened spectrum of gamma photons emitted due to the annihilation of positrons exclusively with 1s electrons of carbon. The width of the extracted Doppler-broadened gamma spectrum has been found to be consistent with the expected broadening of the annihilation gamma spectrum due to the momentum of the 1s electrons in carbon.