Using thermal boundary conditions to engineer the quantum state of a bulk magnet

preprint2014arXivOpen access

Abstract

The degree of contact between a system and the external environment can alter dramatically its proclivity to quantum mechanical modes of relaxation. We show that controlling the thermal coupling of cubic centimeter-sized crystals of the Ising magnet LiHoxY1−xF4LiHo_xY_{1-x}F_4 to a heat bath can be used to tune the system between a glassy state dominated by thermal excitations over energy barriers and a state with the hallmarks of a quantum spin liquid. Application of a magnetic field transverse to the Ising axis introduces both random magnetic fields and quantum fluctuations, which can retard and speed the annealing process, respectively, thereby providing a mechanism for continuous tuning between the destination states. The non-linear response of the system explicitly demonstrates quantum interference between internal and external relaxation pathways.

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