The SrTiO3_3 displacive transition revisited by Coherent X-ray Diffraction

preprint2007arXivOpen access

Abstract

We present a Coherent X-ray Diffraction study of the antiferrodistortive displacive transition of SrTiO3_3, a prototypical example of a phase transition for which the critical fluctuations exhibit two length scales and two time scales. From the microbeam x-ray coherent diffraction patterns, we show that the broad (short-length scale) and the narrow (long-length scale) components can be spatially disentangled, due to 100 μμm-scale spatial variations of the latter. Moreover, both components exhibit a speckle pattern, which is static on a ∼\sim10 mn time-scale. This gives evidence that the narrow component corresponds to static ordered domains. We interpret the speckles in the broad component as due to a very slow dynamical process, corresponding to the well-known \emph{central} peak seen in inelastic neutron scattering.

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