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The Excitation Ladder of Cavity Polaritons

Multidimensional coherent spectroscopy directly unravels multiply excited states that overlap in a linear spectrum. We report multidimensional coherent optical photocurrent spectroscopy in a semiconductor polariton diode and explore the excitation ladder of cavity polaritons. We measure doubly and triply avoided crossings for pairs and triplets of exciton-polaritons, demonstrating the strong coupling between light and dressed doublet and triplet semiconductor excitations. These results demonstrate that multiply excited excitonic states strongly coupled to a microcavity can be described as two coupled quantum-anharmonic ladders.

preprint2020arXivOpen access
Travis M. AutryGaël NardinChristopher L. SmallwoodKevin SilvermanDaniele BajoniAristide LemaîtreSophie BouchouleJacqueline BlochSteven Cundiff
cond-mat.mes-hallcond-mat.quant-gas
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Open access9 authors2 topics
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Travis M. AutryGaël NardinChristopher L. SmallwoodKevin SilvermanDaniele BajoniAristide LemaîtreSophie BouchouleJacqueline BlochSteven Cundiff

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