Temperature evolution of the effective magnetic anisotropy in the MnCr2_2O4_4 spinel

preprint2014arXivOpen access

Abstract

In this work we present a study of the low temperature magnetic phases of polycrystalline MnCr2_2O4_4 spinel through dc magnetization and ferromagnetic resonance spectroscopy (FMR). Through these experiments we determined the main characteristic temperatures: TC_C ∼\sim41 K and TH_H ∼\sim18 K corresponding, respectively, to the ferrimagnetic order and to the low temperature helicoidal transitions. The temperature evolution of the system is described by a phenomenological approach that considers the different terms that contribute to the free energy density. Below the Curie temperature the FMR spectra were modeled by a cubic magnetocrystalline anisotropy to the second order, with K1K_1 and K2K_2 anisotropy constants that define the easy magnetization axis along the <110> direction. At lower temperatures, the formation of a helicoidal phase was considered by including uniaxial anisotropy axis along the [1-10] propagation direction of the spiral arrange, with a KuK_u anisotropy constant. The values obtained from the fittings at 5 K are K1K_1=-2.3x104^4 erg/cm3^3, K2K^2=6.4x104^4 erg/cm3^3 and KuK_u=7.5x104^4 erg/cm3^3.

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