Superconductivity at high Tc in neodymium-doped 1111-SrFeAsF system

Polycrystalline Sr1-xNdxFeAsF samples were prepared at various Nd-doping levels using both a stoichiometric mixture of the starting materials and in slight excess amounts of FeAs. Susceptibility and resistivity of the samples were studied down to 4 K revealing a probable coexistence of superconductivity and a magnetic ordering. Temperature dependence of resistivity for all the Nd-doped samples shows the presence of a transition below 15 K most likely originating from the magnetic ordering of Nd moments, while the spin-density-wave anomaly at 175 K survives up to 0.35 Nd-doping. Superconductivity only occurs above 0.40 Nd-doping with onset maximum Tc reaching as high as 52 K.

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