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Paper detail

Strongly driven quantum pendulum of the OCS molecule

We demonstrate and analyze a strongly driven quantum pendulum in the angular motion of stateselected and laser aligned OCS molecules. Raman-couplings during the rising edge of a 50-picosecond laser pulse create a wave packet of pendular states, which propagates in the confining potential formed by the polarizability interaction between the molecule and the laser field. This wave-packet dynamics manifests itself as pronounced oscillations in the degree of alignment with a laser-intensity dependent period.

preprint2014arXivOpen access
S. TrippelT. MullinsN. L. M. MüllerJ. S. KienitzJ. J. OmisteH. StapelfeldtR. González-FérezJ. Küpper
physics.comp-phphysics.chem-phquant-ph
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S. TrippelT. MullinsN. L. M. MüllerJ. S. KienitzJ. J. OmisteH. StapelfeldtR. González-FérezJ. Küpper

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