Strongest Magnetically Induced Transitions in Alkali Metal Atoms with nuclear spin 3/23/2

preprint2021arXivOpen access

Abstract

The probabilities of atomic transitions Fe−Fg=±2F_e - F_g = \pm 2 between a ground FgF_g and an excited FeF_e level of D2D_2 line of any alkali metal atom are zero when no external magnetic field is applied. In an external magnetic field in the range 0.1−30.1 - 3 kG, the probabilities of these transitions called magnetically induced (MI) are highly modified. For these MI transitions, we have previously exhibited the following rule: the probabilities of MI transitions with ΔF=+2ΔF = +2 are maximal when using σ+σ^+-polarized laser radiation, while the probabilities of MI transitions with ΔF=−2ΔF = -2 are maximal when using σ−σ^--polarized laser radiation. This difference has been termed Type 1 Magnetically Induced Circular Dichroism (MCD1). It is demonstrated for the first time that for alkali atoms with a nuclear spin I=3/2I=3/2 (87Rb^{87}\text{Rb}, 39K^{39}\text{K},23Na^{23}\text{Na}, 7Li^7\text{Li}) in magnetic fields >100> 100 G, the probability of the strongest σ+σ^+ MI transition of the group Fg=1→Fe=3′F_g = 1 \rightarrow F_e = 3' (transition ∣1,−1⟩→∣3′,0′⟩\ket{1,-1}\rightarrow\ket{3',0'}) is about 4 times higher than the probabilities of the strongest MI σ−σ^--transitions ∣1,−1⟩→∣3′,−2′⟩\ket{1,-1}\rightarrow\ket{3',-2'} and ∣2,+1⟩→∣0′,0′⟩\ket{2,+1}\rightarrow \ket{0',0'}. These properties make the σ+σ^+ MI transition ∣1,−1⟩→∣3′,0′⟩\ket{1,-1}\rightarrow\ket{3',0'} an interesting candidate for the study of magneto-optical processes in strong magnetic fields.

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