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Paper detail

Strictly Non-Adiabatic Quantum Control of the Acetylene Dication Using an Infrared Field

We demonstrate the existence of a strictly non-adiabatic control pathway in deprotonation of the acetylene dication. This pathway is identified experimentally by measuring a kinetic energy shift in an ion coincidence experiment. We use a TDSE simulation to identify which properties most strongly affect our control. We find that resonant control around conical intersections is limited by the speed of non-adiabatic dynamics.

preprint2020arXivOpen access
Chelsea Liekhus-SchmaltzXiaolei ZhuGregory A. McCrackenJames P. CryanTodd MartinezPhilip H. Bucksbaum
physics.chem-phquant-ph
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Chelsea Liekhus-SchmaltzXiaolei ZhuGregory A. McCrackenJames P. CryanTodd MartinezPhilip H. Bucksbaum

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