Spin resonance in the superconducting state of Li1−x_{1-x}Fex_{x}ODFe1−y_{1-y}Se observed by neutron spectroscopy

preprint2016arXivOpen access

Abstract

We have performed inelastic neutron scattering measurements on a powder sample of the superconductor lithium iron selenide hydroxide Li1−x_{1-x}Fex_{x}ODFe1−y_{1-y}Se (x≃0.16,y≃0.02x \simeq 0.16, y \simeq 0.02, Tc=41T_{\rm c} = 41\,K). The spectrum shows an enhanced intensity below TcT_{\rm c} over an energy range 0.64×2Δ<E<2Δ0.64\times2Δ< E < 2Δ, where ΔΔ is the superconducting gap, with maxima at the wave vectors Q1≃1.46Q_1 \simeq 1.46\,Å−1^{-1} and Q2≃1.97Q_2 \simeq 1.97\,Å−1^{-1}. The behavior of this feature is consistent with the spin resonance mode found in other unconventional superconductors, and strongly resembles the spin resonance observed in the spectrum of the molecular-intercalated iron selenide, Li0.6_{0.6}(ND2_{2})0.2_{0.2}(ND3_{3})0.8_{0.8}Fe2_{2}Se2_{2}. The signal can be described with a characteristic two-dimensional wave vector (π,0.67π)(π, 0.67π) in the Brillouin zone of the iron square lattice, consistent with the nesting vector between electron Fermi sheets.

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