Spin-Phonon coupling in Y2_2NiMnO6_6 double perovskite probed by Raman spectroscopy

preprint2013arXivOpen access

Abstract

We performed Raman spectroscopy measurements under temperature changes from 10 K up to 850 K to probe the phonon-spin coupling in Y2_2NiMnO6_6. The spin-phonon coupling was observed as a softening of the stretching mode, indicating this phonon stabilizes the magnetic interaction. The result indicates the rare earth ionic radius in Re2_2NiMnO6_6 double perovskites is not the unique parameter influencing the spin-coupling magnitude.

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