Abstract

We demonstrate photodissociation of BeH+^+ ions within a Coulomb crystal of thousands of 9^9Be+^+ ions confined in a Penning trap. Because BeH+^+ ions are created via exothermic reactions between trapped, laser-cooled Be+^+(2P3/2^2\text{P}_{3/2}) and background H2_2 within the vacuum chamber, they represent a major contaminant species responsible for infidelities in large-scale trapped-ion quantum information experiments. The rotational-state-insensitive dissociation scheme described here makes use of 157 nm photons to produce Be+^+ and H as products, thereby restoring Be+^+ ions without the need for reloading. This technique facilitates longer experiment runtimes at a given background H2_2 pressure, and may be adapted for removal of MgH+^+ and AlH+^+ impurities.

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