Production of rovibronic ground state RbCs molecules via two-photon cascade decay

We report the production of ultracold RbCs molecules in the rovibronic ground state, i.e., $X^1Σ^+ (v=0, J=0)$, by short-range photoassociation to the $2^3Π_{0}$ state followed by spontaneous emission. We use narrowband depletion spectroscopy to probe the distribution of rotational levels formed in the $X ^1Σ^+(v=0)$ state. We conclude, based on selection rules, that the primary decay route to $X ^1Σ^+(v=0)$ is a two-step cascade decay that leads to as much as $33\%$ branching into the $J=0$ rotational level. The experimental simplicity of our scheme opens up the possibility of easier access to the study and manipulation of ultracold heteronuclear molecules in the rovibronic ground state.

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