Pressure-enhanced superconductivity in Eu3_3Bi2_2S4_4F4_4

preprint2014arXivOpen access

Abstract

The pressure effect on the newly discovered charge-transferred BiS2_2-based superconductor, Eu3_3Bi2_2S4_4F4_4, with a TcT_c of 1.5 K at ambient pressure, is investigated by transport and magnetic measurements. Accompanied with the enhancement of metallicity under pressures, the onset superconducting transition temperature increases abruptly around 1.0 GPa, reaching ∼\sim10.0 K at 2.26 GPa. AC magnetic susceptibility measurements indicate that a new superconducting phase with a higher TcT_c emerges and dominates at high pressures. In the broad pressure window of 0.68 GPa≤\leqpp≤\leq2.00 GPa, the high-TcT_c phase coexists with the low-TcT_c phase. Hall effect measurements reveal a significant difference in electronic structures between the two superconducting phases. Our work devotes the effort to establish the commonality of pressure effect on the BiS2_2-based superconductors, and also uncovers the importance of electron carrier density in the high-TcT_c phase.

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