Abstract

Concerted experimental and numerical studies of step bunching on vicinal crystal surfaces resulting from step-down electromigration of partially charged adatoms, confirmed the theoretical prediction of scaling dependence of the minimal bunch distance lminl_{\rm min} on the bunch size NN: lmin∼N−γl_{\rm min} \sim N^{-γ}, with γ=2/3γ= 2/3. The value of the so called size-scaling exponent γγ was observed in experiments on vicinal surfaces of semiconducting, metallic, and dielectric materials. Careful theoretical investigations and numerical calculations predict a second value of γ=1/2γ= 1/2. However, this value is still not been reported from experiments. And we report here experimental observation of step bunching in the universality class relative to γ=1/2γ= 1/2. This is achieved by monitoring step flow during sublimation of Si(111)-vicinals heated by a direct step-down current at ~1200∘^\circC. In the experiment we also measure other characteristic for the bunching quantities, such as the mean total number of steps in the bunch NN and the mean bunch width WW. We then compare our findings with published experimental and numerical data to arrive at a theoretically consistent framework in terms of universality classes. The ultimate benefit of our study is not only to advance fundamental knowledge but also to provide further guidance for bottom-up synthesis of vicinal nanotemplates.

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